Nonthermal fragmentation of C60
نویسندگان
چکیده
منابع مشابه
Ultrafast excitation, ionization and fragmentation of C60
The C60 fullerenes are fascinating objects and even many years after their discovery the photo-physics of C60 is still full of surprises. With their well defined, highly symmetric structure the fullerenes are challenging model systems and examples of an interface between atoms or small molecules and the solid state. The 60 delocalized π electrons in the C60 fullerene give rise to interesting bu...
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The sequential absorption of multiple infrared (IR) photons by isolated gas-phase species can lead to their dissociation and/or ionization. Using the newly constructed "Free-Electron Laser for IntraCavity Experiments" (FELICE) beam line at the FELIX facility, neutral C(60) molecules have been exposed to an extremely high number (approximately 10(23)) of photons/cm(2) for a total time duration o...
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The radiation-induced fragmentation of the C60 fullerene was investigated by the tight-binding electron-ion dynamics simulations. In intense laser field, the breathing vibrational mode is much more strongly excited than the pentagonal-pinch mode. The fragmentation effect was found more remarkable at long wavelength λ≥800 nm rather than the resonant wavelengths due to the internal laser-induced ...
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Absolute cross sections have been measured for the first time for H+-impact ionization and fragmentation of C60 at proton energies ranging from 0.2 to 2.0 MeV. The cross sections were in fairly good agreement with other electron-impact data in the high-velocity region, indicating that the charge transfer is negligible in the present energy range. Theoretical cross sections for plasmon excitatio...
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ژورنال
عنوان ژورنال: Chemical Physics Letters
سال: 2002
ISSN: 0009-2614
DOI: 10.1016/s0009-2614(01)01453-1